A method for generating two delayed pulses, in particular in terahertz spectroscopy and/or in pump-probe experiments, with the following method steps:
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1. A method for generating two delayed pulses, the method comprising the following method steps:
generating a pulsed beam using a beam source;
dividing the pulsed beam, wherein a first partial beam contains a first pulse and a second partial beam contains a second pulse;
directing the two pulses onto a respective target area, wherein the first pulse directly reaches a first target area and the second pulse reaches a second target area after covering a delay path;
using the two pulses in one or more of a terahertz spectroscopy experiment and a pump-probe experiment, wherein a time delay of the two pulses in the respective target area is adjusted by means of a pulse repetition rate of the pulsed beam in said one or more of said terahertz spectroscopy experiment and said pump-probe experiment.
23. A method for generating two delayed pulses, the method comprising the following method steps:
generating a pulsed beam using a beam source;
dividing the pulsed beam to form a first partial beam and a second partial beam, wherein said first partial beam comprises a first pulse and said second partial beam comprises a second pulse;
providing a first dipole antenna and a second dipole antenna, said first partial beam being directed to said first dipole antenna, said second partial beam being directed to said second dipole antenna, said second pulse reaching said second dipole antenna after covering a delay path;
generating a terahertz pulse based on said first partial beam;
irradiating a sample with said terahertz pulse;
detecting an electromagnetic pulse with said second dipole antenna after said sample is irradiated with said terahertz pulse, wherein a time delay of said first pulse and said second pulse is adjusted by means of an adjustable pulse repetition rate of the pulsed beam.
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This application is a United States National Phase application of International Application PCT/DE2009/000662 and claims the benefit of priority under 35 U.S.C. §119 of German patent application DE 10 2008 026 484.9 filed Jun. 3, 2008, the entire contents of which are incorporated herein by reference.
The present invention relates to a method for generating two delayed pulses, in which a time delay can be achieved without the use of mechanical parts and in which, in particular, the time delay can be varied in particular in terahertz spectroscopy and/or in pump-probe experiments, with the following method steps:
It is known to use a femtosecond laser in a method in order to activate, using the optical pulses thereof, a photoconductive dipole antenna. In the dipole antenna the laser pulses generate free charge carriers, which are accelerated by an external electrical field. The accelerated charge carriers, in the form of a short current pulse, form the source for an electromagnetic pulse radiated into the space. The electromagnetic pulses generated in this manner may, for example, be used for investigating material, these being used in turn, for example, for monitoring during the production processes of plastics material products or to analyze material. The generation of two time delayed pulses is also the basis for further fields of application such as pump-probe methods, optical tomography, interferometric measurements etc.
These methods are most widespread in the form where a pulsed beam is generated using a beam source, in particular a laser. This beam is divided into a first partial beam with a first pulse and a second partial beam with a second pulse and the pulses are then directed into a target. In this case, one of the two pulses covers a path which is different from the second pulse. This delay path can be realized in the most varied ways, such as, for example, by a mirror, which opposes a second mirror, the spacing of the two mirrors being controllable by means of a precise mechanism or an electronic system. An injected, pulsed beam, in a structure of this type, can cover an adjustable path, which is called a delay path. This path is used to adjust the time delay from a pulse decoupled before this delay path. In this case, a main problem consists in permanently adjusting the mechanical arrangement of the delay path and it is known from constructional systems in this regard that they frequently have to be readjusted.
It is furthermore known from the prior art to configure a delay path for optical signals with a decoupling mirror, which has a spirally curved mirror face. DE 10 2005 011 045 A1 in this regard shows a mirror face with a spiral curvature, the radius changing with the change in the angle of rotation. If a mirror of this type is installed in a corresponding arrangement, the delay path can be changed by rotating the mirror. The mirror body, for this purpose, has two mirror faces, which are arranged symmetrically with respect to a center point, each partial face, starting with an increasing radius, running from a minimum radius through to a maximum radius. Similar problems are produced here as in the previously mentioned prior art in that a mechanism, in this case a rotary mechanism, is required to adjust the delay path, which has to be very precise, and in that the delay path is limited with regard to its variability depending on the radius.
In the conventional method, in particular in the method described above to generate time delayed pulses, the time delay is coupled to the length of the delay path. A limitation of the time delay is thereby produced in that the length of the delay path is limited by the size of the structure. Because of the mechanisms used and the component geometries used, the variability of the delay paths in constructional systems of this type is also very limited. With regard to the delay paths used, problems are also produced with regard to the readjustment and imprecisions due to vibrations at the structure, as with longer optical path lengths covered, the lateral deviations in the sense of the beam laws increase proportionally thereto.
Proceeding from this prior art, the object of the present invention is to provide a method for generating delayed pulses, with which the drawbacks to be found in the prior art can be overcome and, in particular, a simplified adjustment is made possible.
This object is achieved according to the invention by a method in which a time delay of the two pulses in the respective target area is adjustable by means of a pulse repetition rate of the pulsed beam.
The method of the invention thus basically comprises the following disclosed method steps:
Consequently, two or more pulses can be directed into a respective target area, it being possible on the basis of the proposed method to adjust the time interval between the impinging of the individual pulses in the respective target area by means of the repetition rate. There is no restriction of any type to the effect that the time delay is limited, for example, by a finite delay path. It is therefore now in particular possible in terahertz technology, to generate two terahertz pulses which have a very large time interval with respect to one another. Avoidance of the adjustment of moveable parts during the method facilitates the work in that it is substantially more seldom necessary to readjust the structure, a more precise operation afflicted by fewer errors of a device of this type being produced because of the reduction in number of moveable parts. The use of glass fiber cables for guiding the laser beam or the pulsed signal allows a very stable structure, it also being possible to achieve simpler assembly for products which relate to a structure for using a proposed method.
It is provided in a preferred embodiment that the pulsed beam impinges on a beam splitter, in particular on a fiber coupler and is divided into a first partial beam with a first pulse and a second partial beam with a second pulse. The beam splitter mentioned here may be configured as semi-permeable mirrors for a so-called free beam structure, a possibility also existing for generating a plurality of pulses by the use of a plurality of partially permeable beam splitters. In fiber-coupled systems, a fiber coupler is a possibility by way of example for the beam splitter in order to separate the pulsed beam into a first fiber, which contains a first partial beam with a first pulse, and into a second fiber, which contains a second partial beam with a second pulse, it being possible to carry this out with all types of light guides.
It is provided in a further configuration that the first and the second pulse come from the same pulse of the pulsed signal, a measurement of the pulse only being thought of by way of example. It may furthermore be provided that the first pulse and the second pulse originate from different pulses of the pulsed signal in order to achieve a time delay of the electromagnetic pulses generated during the production, for example, of electromagnetic pulses, which originate from activated dipole antennae. Thus, depending on the required time delay, a corresponding first and second pulse from the pulsed signal can be used. To use the pulses for pulse measurement, applications in the area of ultra-short time physics are thought of by way of example, in order to overlay femtosecond or attosecond pulses, for example, by means of cross correlation and to integrate them in a slow photodetector via the signal in order to come to conclusions about their form and to check the signal quality.
According to a further embodiment of the invention, the first pulse is directed by means for beam deflection into a target area. This may take place in a simple manner, for example by means of a mirror or in a free beam structure. Analogously to this, in a fiber-coupled system, a signal can be deflected by a correspondingly formed light guide. In order to adjust the beam deflection or adapt it to the use, further means for adjustment are thought of. Likewise, further optical components and/or means for beam deflection can also be inserted in a further use according to requirements.
According to a preferred embodiment, the second pulse is directed by means for beam deflection into a target area, it being provided that the pulse covers a path which is different from the first pulse, in particular a longer delay path. A delay path, in particular, means a longer path in comparison to the first pulse, in this case. These can be any means for beam deflection. Mirrors or glass fibers are preferably in turn used. The length of the delay path is implemented, by way of example, with a fixed length, which may be changed, however, for adjustment and also for continuing pulse generation. For precise calculation of the time delay or to adjust it, it may be necessary for the first and second pulse to cover a different path.
Moreover, it is particularly preferred for the delay path, which the second pulse covers to have a constant length, which is different from zero, in order to keep the time delay of the first and the second pulse substantially constant in the respective target area. Moreover, it is found that the time delay is variably adjustable in principle by means of the repetition rate. The delay path, which the second pulse covers, can likewise, in particular in terahertz spectroscopy, be realized by a longer glass fiber in comparison to the glass fiber, which guides the first pulse.
According to a particularly preferred configuration, the delay path is configured as an arrangement to compensate the pulse widening, by dispersion in a glass fiber or else in air. In this case, it is possible to also provide further optical elements in the delay path, which can change the pulse not only in relation to its form and duration.
In order to adjust the time delay of the two pulses in the respective target area by means of the repetition rate of the pulsed signal, it is particularly preferably provided that the length of the delay path be kept constant and only be adapted for adjustment. This produces a substantial improvement to constructional systems in this regard as the time delay is not carried out by means of the change in the length of the delay path and therefore the change in the delay path does not lead to errors, either.
According to a further configuration of the invention it may be provided that the time delay of the two pulses in the respective target is produced from the length of the delay path, the speed of propagation of the pulses, the pulse repetition rate and a factor for the number of pulses of the laser source, which lies between the pulses generating the first and the second pulse. In this case, the length of the delay path takes into account the length from the beam splitter to the first impingement point, the length from the beam splitter to a possibly present means for beam deflection and the length from a possibly present means for beam deflection to a second impingement point.
According to a most simple implementation of the structure with a respective light guide for the first and the second partial beam or pulse, only the length difference of the two light guides can be regarded as the delay path. In this embodiment, using the speed of propagation, the ratio of the refraction index and the vacuum light speed for the material has to be taken into account, through which the two signals are guided, wherein no limitation should be produced to the effect that different light guides are also used to guide the first and the second pulse. The factor for the number of pulses of the laser source, which lie between the pulses generating the first and the second pulse, is produced, in the simplest case, from a listed numbering of the pulses, which leave the pulsed beam source.
It may furthermore be provided that the repetition rate is determined by means of photo sensors and used to determine the time delay when the length of the delay path is known. Although the repetition rate can also be determined by means of the length of the resonator in the laser, it may, however, be more favorable to decouple the signal and to determine the repetition rate by means of a photo sensor. This may take place by means of any optical elements which are used to allocate an electrical signal to a light signal, the measurement of intensities then, by way of example, being reduced to a measurement of voltages.
According to a further preferred embodiment of the method according to the invention it may be provided that a variation of the time delay of the first and second pulse in the respective target area is achieved by means of varying the pulse repetition rate. Thus, for example, relaxation processes can be resolved with respect to time to thus come to conclusions about time-dependent processes within the subject investigated. Furthermore, it may additionally be provided that a corresponding investigation is repeatedly carried out under the same conditions with a rigidly adjusted repetition rate with a constant time interval of the two pulses, as a specific result can thus be determined more precisely. The concluding use of the two pulses in the respective target area is particularly preferably provided to generate and/or detect an electromagnetic pulse. This is to be attributed to a use in terahertz physics, a dipole antenna being exposed to a laser pulse and the generated free charge carriers in an electrical field being accelerated and thus generating a terahertz pulse. The application of the time-delayed pulses is very diverse in principle and can be used, in particular, to measure processes on very small timescales. In this case, it is now possible to carry out a continuous measurement of various states of a system which are in a time sequence, by means of the adjustment of the time delay in a large area.
The various features of novelty which characterize the invention are pointed out with particularity in the claims annexed to and forming a part of this disclosure. For a better understanding of the invention, its operating advantages and specific objects attained by its uses, reference is made to the accompanying drawings and descriptive matter in which preferred embodiments of the invention are illustrated.
In the drawings:
Referring to the drawings in particular,
The calculation of the pulse delay by changing the repetition rate will be described below.
The time interval τ of two consecutive pulses of the laser with the repetition rate R corresponds to τ0=1/R
In general, the time interval τ of a pulse I(i)=i from the pulse I(i+a)=i+a with the pulse interval ΔI=I(i+a)−I(i)=a can be described as follows.
τ=ΔI·τ0=ΔI/R
The running time t of an electromagnetic wave through a medium with the refraction index n and a path l passed through at the vacuum light speed c0 is
t=l·n/c0.
If the time difference Δt of the impingement time of a pulse I(i) is observed in the two partial beams, this is composed of the time required to cover the paths beam splitter-impingement point 1 at t1, beam splitter-means for deflection of the beam at tv and means for deflecting the beam-impingement point 2 at t2 and produces
Δt=t2+tv−t1,
wherein this at t1=constant and t2=constant and tv=variable corresponds to the conventional delay path.
Therefore the interval between the impingement time of a pulse I(i)=i in the first partial beam and of a pulse I(i+a)=i+a in the second partial beam at ΔI=a is
Δτ=t2+tv−t1−τ.
Therefore, for the second interval
Δτ=l2·n2/c0+lv·nv/c0+l1·n1/c0−ΔI/R.
is produced.
Therefore, taking into account all the paths and refraction indices while observing two different pulses, the pulse delay can be varied by changing the repetition rate.
In addition, the variation area of the pulse delay from the repetition rate may be varied between Rmin and Rmax. This produces
Δτvar=ΔI·(1/Rmin−1/Rmax)
While specific embodiments of the invention have been described in detail to illustrate the application of the principles of the invention, it will be understood that the invention may be embodied otherwise without departing from such principles.
Koch, Martin, Hochrein, Thomas Eugen, Krumbholz, Norman
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